Antisolvent precipitation of hydrophobic functionalized multiwall carbon nanotubes in an aqueous environment

Desai, C; Addo Ntim, S; Mitra, S

HERO ID

955029

Reference Type

Journal Article

Year

2012

Language

English

PMID

22142999

HERO ID 955029
In Press No
Year 2012
Title Antisolvent precipitation of hydrophobic functionalized multiwall carbon nanotubes in an aqueous environment
Authors Desai, C; Addo Ntim, S; Mitra, S
Journal Journal of Colloid and Interface Science
Volume 368
Issue 1
Page Numbers 115-120
Abstract The possibility of antisolvent precipitation of hydrophobic, organic soluble functionalized carbon nanotubes (f-CNTs), where water acts as an antisolvent is presented. Octadecylamine functionalized multiwall carbon nanotubes (MWCNT-ODA) was used as the model compound and was found to form highly stable dispersions in different water/solvent systems, and the particle sizes ranged from 170 to 400nm. Colloidal behavior was studied using dynamic light scattering and particle aggregation was found to increase with the addition of electrolytes, with tetrahydrofuran (THF) and ethanol showing the maximum effect. The aggregation behavior of the antisolvent precipitated system did not follow the conventional Derjaguin-Landau-Verwey-Overbeek (DLVO) theory, which was different from what has been reported previously for hydrophilic, water soluble f-CNTs. Based on this study, it is evident that hydrophobic f-CNTs are potential water pollutants.
Doi 10.1016/j.jcis.2011.11.019
Pmid 22142999
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Dupe Override No
Is Public Yes
Language Text English
Is Qa No