Estimating fine particulate matter component concentrations and size distributions using satellite-retrieved fractional aerosol optical depth: part 2--a case study

Liu, Y; Koutrakis, P; Kahn, R; Turquety, S; Yantosca, RM

HERO ID

98197

Reference Type

Journal Article

Year

2007

Language

English

PMID

18069459

HERO ID 98197
In Press No
Year 2007
Title Estimating fine particulate matter component concentrations and size distributions using satellite-retrieved fractional aerosol optical depth: part 2--a case study
Authors Liu, Y; Koutrakis, P; Kahn, R; Turquety, S; Yantosca, RM
Journal Journal of the Air and Waste Management Association
Volume 57
Issue 11
Page Numbers 1360-1369
Abstract We use the fractional aerosol optical depth (AOD) values derived from Multiangle Imaging Spectroradiometer (MISR) aerosol component measurements, along with aerosol transport model constraints, to estimate ground-level concentrations of fine particulate matter (PM2.5) mass and its major constituents in the continental United States. Regression models using fractional AODs predict PM2.5 mass and sulfate (SO4) concentrations in both the eastern and western United States, and nitrate (NO3) concentrations in the western United States reasonably well, compared with the available ground-level U.S. Environment Protection Agency (EPA) measurements. These models show substantially improved predictive power when compared with similar models using total-column AOD as a single predictor, especially in the western United States. The relative contributions of the MISR aerosol components in these regression models are used to estimate size distributions of EPA PM2.5 species. This method captures the overall shapes of the size distributions of PM2.5 mass and SO4 particles in the east and west, and NO3 particles in the west. However, the estimated PM2.5 and SO4 mode diameters are smaller than those previously reported by monitoring studies conducted at ground level. This is likely due to the satellite sampling bias caused by the inability to retrieve aerosols through cloud cover, and the impact of particle hygroscopicity on measured particle size distributions at ground level.
Doi 10.3155/1047-3289.57.11.1360
Pmid 18069459
Wosid WOS:000250768400008
Is Certified Translation No
Dupe Override No
Is Public Yes
Language Text English
Is Qa No