TIME-RESOLVED EFFECTS OF AN ELECTRIC-FIELD IN RECOMBINATION FLUORESCENCE

Borovkov, VI; Anishchik, SV; Anisimov, OA

HERO ID

4969113

Reference Type

Journal Article

Year

1995

HERO ID 4969113
In Press No
Year 1995
Title TIME-RESOLVED EFFECTS OF AN ELECTRIC-FIELD IN RECOMBINATION FLUORESCENCE
Authors Borovkov, VI; Anishchik, SV; Anisimov, OA
Journal High Energy Chemistry
Volume 29
Issue 6
Page Numbers 401-406
Abstract Quenching of the recombination fluorescence by an external electric field was investigated in hexane, tetradecane, and squalane solutions of p-terphenyl and 2.5-diphenyloxazole irradiated with X-rays. The kinetics of the recombination fluorescence I(E, t) was measured in a nanosecond time scale and the quenching-efficiency curves Q(E, t) = 1 - I(E, t)/I(0, t) were plotted. The dependence Q(E, t) was shown to have the specific character Q(E, t) = f(pt), where p = AE(2)D/r(c)(2). Here A is a constant dependent on the initial-distance distribution function of the charges, E is the electric field strength, D is a mutual diffusion coefficient of the recombining ions, and r(c), is the Onsager radius. The quadratic dependence of the parameter p on the electric field strength was shown to be a consequence of the diffusion-controlled reaction of ion recombination.
Wosid WOS:A1995TJ96900007
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Dupe Override No
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