A novel approach to fluorinated polyurethane by macromonomer copolymerization

Jiang, M; Zhao, XL; Ding, XB; Zheng, ZH; Peng, YX

HERO ID

3859434

Reference Type

Journal Article

Year

2005

Language

English

HERO ID 3859434
In Press No
Year 2005
Title A novel approach to fluorinated polyurethane by macromonomer copolymerization
Authors Jiang, M; Zhao, XL; Ding, XB; Zheng, ZH; Peng, YX
Journal European Polymer Journal
Volume 41
Issue 8
Page Numbers 1798-1803
Abstract For the first time, through macromonomer radical copolymerization, a novel fluorinated polyurethane (FPU) was synthesized based on partly acrylate-endcapped polyurethane macromonomers with hexafluorobutyl acrylate (HFBA). Partly acrylate-endcapped polyurethane (PU) macromonomers were synthesized using isophronediisocyanate (IPDI), dimethylol propionic acid (DMPA), polyethylene adipate glycols (PEA) etc. The novel fluorinated polymer, which bore PU side chains and fluorinated side chains, was confirmed by F-19 NMR spectroscopy, X-ray photoelectron spectroscopy (XPS), elemental analysis, scanning electron spectroscopy (SEM) etc. Copolymerization of polyurethane macromonomers with hexafluorobutyl acrylate (HFBA) was briefly investigated. The surface tension of FPU solution was measured and showed sharply decrease compared to that of pure polyurethane. Results from SEM showed a uniform size distribution of phase micro-domains on the fracture surface of FPU. (c) 2005 Elsevier Ltd. All rights reserved.
Doi 10.1016/j.eurpolymj.2005.02.013
Wosid WOS:000230638600012
Is Certified Translation No
Dupe Override No
Comments Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-20344380155&doi=10.1016%2fj.eurpolymj.2005.02.013&partnerID=40&md5=52cea860f6607f17248f2078f4d02dc6
Is Public Yes
Language Text English
Keyword macromonomers; acrylate-endcapped; copolymerization; fluorinated polyurethane; radical polymerization