N-benzoyl-1,5-benzothiazepine and its S-oxide as vasopressin receptor ligands: insight into the active stereochemistry around the seven-membered ring

Yoneda, T; Tabata, H; Tasaka, T; Oshitari, T; Takahashi, H; Natsugari, H

HERO ID

2902177

Reference Type

Journal Article

Year

2015

Language

English

PMID

25774991

HERO ID 2902177
In Press No
Year 2015
Title N-benzoyl-1,5-benzothiazepine and its S-oxide as vasopressin receptor ligands: insight into the active stereochemistry around the seven-membered ring
Authors Yoneda, T; Tabata, H; Tasaka, T; Oshitari, T; Takahashi, H; Natsugari, H
Journal Journal of Medicinal Chemistry
Volume 58
Issue 7
Page Numbers 3268-3273
Abstract The stereochemistry of N-benzoyl-1,5-benzothiazepine and its S-oxide derivatives as vasopressin receptor ligands was examined in detail by freezing the conformation with a methyl group at the C6 or C9 of 1,5-benzothiazepine. It was revealed that the active forms recognized by the receptors are (cis,aS) for 1,5-benzothiazepine (5-7)-II and (cis,1S,aS) (syn) for its S-oxide (8-10)-II. The C9-methyl derivative of 1,5-benzothiazepine S-oxide (10-II) was designed and synthesized, achieving the putative active syn-isomer.
Doi 10.1021/acs.jmedchem.5b00289
Pmid 25774991
Is Certified Translation No
Dupe Override No
Is Public Yes
Language Text English