Influence of carbon support microstructure on the polarization behavior of a polymer electrolyte membrane fuel cell membrane electrode assemblies

Guha, A; Zawodzinski, TA, Jr; Schiraldi, DA

HERO ID

2616173

Reference Type

Journal Article

Year

2010

HERO ID 2616173
In Press No
Year 2010
Title Influence of carbon support microstructure on the polarization behavior of a polymer electrolyte membrane fuel cell membrane electrode assemblies
Authors Guha, A; Zawodzinski, TA, Jr; Schiraldi, DA
Journal Journal of Power Sources
Volume 195
Issue 16
Page Numbers 5167-5175
Abstract The influence of Cr3C2 and VC addition on the microstructure and mechanical properties of WC-Mg composites hot-pressed at 1650 degrees C for 90 min was comprehensively investigated. The grain growth of WC was significantly retarded and the homogeneity of MgO particulate dispersion was effectively improved with the addition of 0.5 wt.% Cr3C2 or 0.5 wt.% VC. The indentation size effect (ISE) on hardness was restrained and the load-independent hardness was increased by doping grain growth inhibitors. Improvements on fracture toughness of hot-pressed samples were also observed due to the refined WC grains and uniformly dispersed MgO particulates. In addition, experimental results demonstrated that Niihara's equation was preferable for estimating the indentation fracture toughness, by comparing the fracture toughness evaluated using the single-edge V-notch beam (SEVNB) method with the values estimated through the Vickers indentation technique. (C) 2013 Elsevier Ltd. All rights reserved.
Doi 10.1016/j.jpowsour.2010.03.006
Wosid WOS:000277868600002
Is Certified Translation No
Dupe Override No
Is Public Yes
Keyword Carbon nanofibers; Vulcan XC-72 carbon; Catalyst support; Support morphology; Membrane electrode assembly