Synthesis and bioactivity of novel coumarin derivatives

Guan, AY; Liu, CL; Li, M; Li, ZN; Zhang, MX; Zhang, H

HERO ID

2530333

Reference Type

Journal Article

Year

2011

Language

English

PMID

22312739

HERO ID 2530333
In Press No
Year 2011
Title Synthesis and bioactivity of novel coumarin derivatives
Authors Guan, AY; Liu, CL; Li, M; Li, ZN; Zhang, MX; Zhang, H
Journal Natural Product Communications
Volume 6
Issue 12
Page Numbers 1917-1920
Abstract A series of coumarin derivatives (6-8) containing (E)-methyl 2-(methoxyimino)-2-phenylacetate, (E)-2-(methoxyimino)-N-methyl-2-phenylacetamide and methyl methoxy(phenyl)carbamate were synthesized from substituted resorcinols (1) and substituted beta-keto esters (2) as starting material via cyclization and condensation reactions. The test results indicated that (E)-methyl 2-{2-[(3-hexyl-4-methyl-coumarin-7-yloxy)methyl]phenyl}-2-(methoxyimino)acetate (6f) was the optimal structure with good fungicidal activity against cucumber grey mold (CGM) giving 100% control at 100 mg L(-1) concentration, much higher than that of coumoxystrobin. Methyl 2-[(3,4-dimethyl-coumarin -7-yloxy)methyl]phenyl(methoxy)carbamate (8a) was another optimal structure with good fungicidal activity against wheat powdery mildew (WPM) showing 100% control at 50 mg L(-1) concentration, at the same level as that of the commercial kresoxim-methyl, and very significantly higher than that of coumoxystrobin (no control against WPM at 400 mg L(-1)).
Doi 10.1177/1934578x1100601232
Pmid 22312739
Wosid WOS:000298445300032
Is Certified Translation No
Dupe Override No
Comments Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-83455224317&doi=10.1177%2f1934578x1100601232&partnerID=40&md5=266e3a5d0c72fc3a5a91fc6fd217fc57
Is Public Yes
Language Text English
Keyword Coumarins; Fungicidal activity; Insecticidal activity; Intermediate derivatization method; Strobilurins; 2 (methoxyimino) n methyl 2 [2 [(4 methylcoumarin 7 yloxy)methyl]phenyl]acetamide; antifungal agent; coumarin derivative; coumoxystrobin; kresoxim methyl; methyl 2 [(3,4 dimethylcoumarin 7 yloxy)methyl]phenyl(methoxy)carbamate; methyl 2 [2 [(3 hexyl 4 methylcoumarin 7 yloxy)methyl]phenyl] 2 (methoxyimino)acetate; unclassified drug; antifungal activity; article; chemical reaction; concentration response; controlled study; cucumber grey mold; cyclization; drug structure; drug synthesis; mould; nonhuman; powdery mildew
Is Peer Review No