Formaldehyde assay by capacitance versus voltage and impedance measurements using bi-layer bio-recognition membrane

Ben Ali, M; Korpan, Y; Gonchar, M; El'skaya, A; Maaref, MA; Jaffrezic-Renault, N; Martelet, C

HERO ID

1578864

Reference Type

Journal Article

Year

2006

Language

English

PMID

16516460

HERO ID 1578864
In Press No
Year 2006
Title Formaldehyde assay by capacitance versus voltage and impedance measurements using bi-layer bio-recognition membrane
Authors Ben Ali, M; Korpan, Y; Gonchar, M; El'skaya, A; Maaref, MA; Jaffrezic-Renault, N; Martelet, C
Journal Biosensors and Bioelectronics
Volume 22
Issue 5
Page Numbers 575-581
Abstract A novel formaldehyde sensitive biosensor based on bacterial formaldehyde dehydrogenase (FDH) as a bio-recognition element has been developed. The bio-recognition membrane had bi-layer architecture and consisted of FDH, cross-linked with albumin, and of the cofactor NAD at a high concentration level (first layer). The second layer was a negatively charged Nafion membrane, which prevented a leakage of negatively charged NAD molecules from the bio-membrane. As transducers, gold electrodes SiO(2)/Si/SiO(2)/Ti/Au and electrolyte-insulator-semiconductor Si/SiO(2) (EIS) structures have been used. Changes in capacitance and impedance properties of the bio-recognition membrane have been used for monitoring formaldehyde concentration in a bulk solution. It has been shown that formaldehyde can be detected within a concentration range from 1 microM to 20mM depending on the type of transduction used, with a detection limit of 1 and 100 microM for gold-based and EIS-based transducers, respectively.
Doi 10.1016/j.bios.2006.01.019
Pmid 16516460
Wosid WOS:000242230800001
Is Certified Translation No
Dupe Override No
Is Public Yes
Language Text English